Abstract:
This work investigates the dynamics of large-scale, ‘wet’ volcanic eruption clouds
generated by the interaction of silicic magma with external water. The primary case
study draws from a detailed record of non-welded pyroclastic deposits from the ~25.4
ka Oruanui eruption of Taupo volcano, New Zealand, one of the largest
phreatomagmatic eruptions documented worldwide. This research uses a three-pronged
approach, integrating results from (i) field observations and textural data, (ii) mesoscale
numerical modeling of volcanic plumes, and (iii) analogue laboratory experiments of
volcanic ash aggregation. This interdisciplinary approach provides a new understanding
of dynamic and microphysical interactions between collapsing and buoyant columns,
and how this behavior controls the large-and small-scale nature of phreatoplinian
eruption clouds.
Stratigraphic field studies examine the styles of dispersal and emplacement of deposits
from several phases of the Oruanui eruption (primarily phases 2, 3, 5, 6, 7 and 8).
Detailed stratigraphic observations and laser diffraction particle size analysis of ash
aggregates in these deposits clarify the evolution of aggregation mechanisms with time
through the relevant eruption phase, and with distance from vent. Deposits of the
wettest phase (3) show the key role of turbulent lofting induced by pyroclastic density
currents in forming aggregates, particularly those with ultrafine ash rims (30-40 vol.%
finer than 10 μm) which are uniquely formed in the ultrafine ash-dominated clouds
above the currents. Drier deposits of phases 2 and 5, which also saw lower proportions
of material emplaced by pyroclastic density currents, contain fewer aggregates that are
related to low water contents in the medial to distal plume. Discovery and
documentation of high concentrations of diatom flora in the Oruanui deposits indicates
efficient fragmentation and incorporation of paleo-lake Taupo sediments during the
eruption. This highlights the potential for incidental contamination of volcanic deposits
with broader implications for correlation of distal tephras and possible contamination of
paleoenvironmental records due to incorporation of diachronous populations of
volcanically-dispersed diatoms.
The impact of extensive surface water interaction on large-scale volcanic eruptions
(>108 kg s-1 magma) is examined by employing the first 2-D large-eddy simulations of
‘wet’ volcanic plumes that incorporate the effects of microphysics. The cloud-resolving
numerical model ATHAM was initialized with field-derived characteristics of the
Oruanui case study. Surface water contents were varied from 0-40 wt.% for eruptions
with equivalent magma eruption rates of c. 1.3 x108 and 1.1 x109 kg s-1. Results confirm
that increased surface water has a pronounced impact on column stability, leading to
unstable column behavior and hybrid clouds resulting from simultaneous ascent of
material from stable columns and pyroclastic density currents (PDCs). Contrary to the
suggestion of previous studies, however, abundant surface water does not systematically
lower the spreading level or maximum height of volcanic clouds, owing to vigorous
microphysics-assisted lofting of PDCs.
Key processes influencing the aggregation of volcanic ash and hydrometeors (airborne
water phases) are examined with a simple and reproducible experimental method
employing vibratory pan agglomeration. Aggregation processes in the presence of hail
and graupel, liquid water (<30 wt.%), and mixed water phases are investigated at temperatures from 18 to -20 °C. Observations from impregnated thin sections, SEM
images and x-ray computed microtomography of these experimental aggregates closely
match natural examples from phreatomagmatic phases of the ~25.4 ka Oruanui and
Eyjafjallajökull (May 2010) eruptions. These experiments demonstrate that the
formation of concentric, ultrafine rims comprising the outer layers of rim-type
accretionary lapilli requires recycled exposure of moist, preexisting pellets to regions of
volcanic clouds that are relatively dry and dominated by ultrafine (<31 μm) ash. This
work presents the first experimentally-derived aggregation coefficients that account for
changing liquid water contents and sub-zero temperatures, and indicates that dry
conditions (<10 wt.% liquid) promote the strongly size-selective collection of sub-31
μm particles into aggregates (given by aggregation coefficients >1). These quantitative
relationships may be used to predict the timescales and characteristics of aggregation,
such as aggregate size spectra, densities and constituent particle size characteristics,
when the initial size distribution and hydrometeor content of a volcanic cloud are
known.
The integration of numerical modeling, laboratory experimentation and field data lead
to several key conclusions. (1) The importance of the microphysics of ash-water
interactions in governing the eruption cloud structure, boosting the dispersal power of
the cloud and controlling aggregate formation in response to differing water contents
and eruption rates. (2) Recognition of the contrasting roles of differential aggregation
versus cloud grain size in controlling the formation and nature of aggregate particles,
notably those with characteristic ultrafine outer rims. (3) The importance of pyroclastic
density currents as triggers for convection and aggregation processes in the eruption
cloud.